This should fit smoothers to all of your blocks. Check "Standardize X" as well and press OK. Release Ctrl now and type 0.002 for the smoothness value (this value seemed to work well for me). Holding Ctrl, click the red-arrow icon next to "Bivariate Fit of 9 by Voltage" > Flexible > Fit Spline > Other.Do Fit Y by X with Voltage in X, and all the other columns in Y.Get rid of columns corresponding to block 0 through 8 (these are the lower moded ones you said you didn't want to look at).Do a table split on Time, split by Block, Group by Voltage - Result is Table 2 attached.Hope this is clear enough to follow along. There's a few splits and stacks to get the data in the right format so we can do the spline fitting, predictions for new values of Voltage, and then compute the standard deviations.
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